338 citations · 628 across the 8 of their papers we have counts for
8 papers
Entangled-photon time- and frequency-resolved optical spectroscopy
Raul Alvarez-Mendoza, Lorenzo Uboldi, Ashley Lyons +3
Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders o…
Disentangling Dynamical Quantum Coherences in the Fenna-Matthews-Olson Complex
Hong-Guang Duan, Ajay Jha, Lipeng Chen +6
In the primary step of light-harvesting, the energy of a photon is captured in antenna chlorophyll as an exciton. Its efficient conversion to stored chemical potential occurs in th…
Quieting a noisy antenna reproduces photosynthetic light harvesting spectra
Trevor B. Arp, Jed Kistner-Morris, Vivek Aji +3
Photosynthesis is remarkable, achieving near unity light harvesting quantum efficiency in spite of dynamic light conditions and noisy physiological environment. Under these adverse…
Unexpectedly large delocalization of the initial excitation in photosynthetic light harvesting
Khadga J. Karki, Junsheng Chen, Atsunori Sakurai +5
Electronic 2D spectroscopy allows nontrivial quantum effects in chemistry and biology to be explored in unprecedented detail. Here, we apply recently developed fluorescence detecte…
Spatially-resolved Fluorescence-detected Two-dimensional Electronic Spectroscopy Probes Varying Electronic Couplings in Photosynthetic Bacteria
Vivek Tiwari, Yassel Acosta-Matutes, Alastair T. Gardiner +2
We present a variation of two-dimensional electronic spectroscopy that is capable of mapping spatially-varying differences in electronic couplings using a correlated map of excitat…
Nature does not rely on long-lived electronic quantum coherence for photosynthetic energy transfer
Hong-Guang Duan, Valentyn I. Prokhorenko, Richard Cogdell +4
During the first steps of photosynthesis, the energy of impinging solar photons is transformed into electronic excitation energy of the light-harvesting biomolecular complexes. The…
Ultrafast Energy Relaxation in Single Light-Harvesting Complexes
Pavel Malý, J. Michael Gruber, Richard J. Cogdell +2
Energy relaxation in light-harvesting complexes has been extensively studied by various ultrafast spectroscopic techniques, the fastest processes being in the sub-100 fs range. At…
Vibronic coupling explains the ultrafast carotenoid-to-bacteriochlorophyll energy transfer in natural and artificial light harvesters
Václav Perlík, Joachim Seibt, Laura J. Cranston +6
The initial energy transfer in photosynthesis occurs between the light-harvesting pigments and on ultrafast timescales. We analyze the carotenoid to bacteriochlorophyll energy tran…