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Mechanistic Modeling of Lipid Nanoparticle Formation for the Delivery of Nucleic Acid Therapeutics
Pavan K. Inguva, Saikat Mukherjee, Pierre J. Walker +13
Nucleic acids such as mRNA have emerged as a promising therapeutic modality with the capability of addressing a wide range of diseases. Lipid nanoparticles (LNPs) as a delivery pla…
Potential of mean force and underscreening of polarizable colloids in concentrated electrolytes
Emily Krucker-Velasquez, Martin Z. Bazant, Alfredo Alexander-Katz +1
This study uses advanced numerical methods to estimate the mean force potential (PMF) between charged, polarizable colloidal particles in dense electrolytes. We observe that when t…
Theory of Cation Solvation and Ionic Association in Non-Aqueous Solvent Mixtures
Zachary A. H. Goodwin, Michael McEldrew, Boris Kozinsky +1
Conventional lithium-ion batteries, and many next-generation technologies, rely on organic electrolytes with multiple solvents to achieve the desired physicochemical and interfacia…
Polar Liquids at Charged Interfaces: A Dipolar Shell Theory
J. Pedro de Souza, Alexei A. Kornyshev, Martin Z. Bazant
The structure of polar liquids and electrolytic solutions, such as water and aqueous electrolytes, at interfaces underlies numerous phenomena in physics, chemistry, biology, and en…
Gelation, Clustering and Crowding in the Electrical Double Layer of Ionic Liquids
Zachary A. H. Goodwin, Michael McEldrew, J. Pedro de Souza +2
Understanding the bulk and interfacial properties of super-concentrated electrolytes, such as ionic liquids (ILs), has attracted significant attention lately for their promising ap…
Dip-coating of bidisperse particulate suspensions
Deok-Hoon Jeong, Michael Ka Ho Lee, Virgile Thiévenaz +2
Dip-coating consists in withdrawing a substrate from a bath to coat it with a thin liquid layer. This process is well-understood for homogeneous fluids, but heterogeneities such as…