5 papers
Using near-flat-band electrons for read-out of molecular spin qubit entangled states
Christian Bunker, Silas Hoffman, Shuanglong Liu +2
While molecular spin qubits (MSQs) are a promising platform for quantum computing, read-out has been largely limited to electron paramagnetic resonance which is often slow and requ…
Floquet Engineering Clock Transitions in Magnetic Molecules
Andrew Cupo, Shuanglong Liu, Silas Hoffman +2
We theoretically study Floquet engineering of magnetic molecules via a time-periodic magnetic field that couples to the emergent total electronic spin of the metal center. By focus…
Dominant spin-spin relaxation mechanism at clock transition of the complex at different concentrations
Xiao Chen, Haechan Park, Silas Hoffman +2
Spin decoherence poses a significant challenge in molecular magnets, with the nuclear spin bath serving as a prominent source. Intriguingly, spin qubits at the clock transition exh…
Accurate crystal field Hamiltonians of single-ion magnets at mean-field cost
Linqing Peng, Shuanglong Liu, Xing Zhang +4
The effective crystal field Hamiltonian provides the key description of the electronic properties of single-ion magnets, but obtaining its parameters from ab initio computation is…
Tuning the Magnetic Anisotropy Energy of MoS-supported Mn complexes by Electric Field: A First-Principles Study
Shuanglong Liu, Adam V. Bruce, Dmitry Skachkov +2
In this work, we examine low-energy adsorption configurations of four dodecanuclear manganese single-molecule magnets [MnO(OCR)(HO)] (Mn), w…