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X-ray diffractive imaging of controlled gas-phase molecules: Toward imaging of dynamics in the molecular frame
Thomas Kierspel, Andrew Morgan, Joss Wiese +25
We report experimental results on the diffractive imaging of three-dimensionally aligned 2,5-diiodothiophene molecules. The molecules were aligned by chirped near-infrared laser pu…
Imaging the Breakdown of Molecular-Frame Dynamics through Rotational Uncoupling
Lucas J. Zipp, Adi Natan, Philip H. Bucksbaum
We demonstrate the breakdown of molecular-frame dynamics induced by the uncoupling of molecular rotation from electronic motion in molecular Rydberg states. We observe this non-Bor…
Observation of Quantum Interferences via Light Induced Conical Intersections in Diatomic Molecules
Adi Natan, Matthew R Ware, Vaibhav S. Prabhudesai +4
We observe energy-dependent angle-resolved diffraction patterns in protons from strong-field dissociation of the molecular hydrogen ion H. The interference is a characteristi…
Strongly aligned gas-phase molecules at Free-Electron Lasers
Thomas Kierspel, Joss Wiese, Terry Mullins +27
We demonstrate a novel experimental implementation to strongly align molecules at full repetition rates of free-electron lasers. We utilized the available in-house laser system at…