Nonadiabatic vibrational dynamics of CO on Pt(111) studied with first-principles many-body perturbation theory

Raúl Bombín, Iñaki Fernández Tena, J. Iñaki Juaristi +1

We investigate the nonequilibrium vibrational dynamics of CO adsorbed on Pt(111), a prototypical adsorbate-surface system for ultrafast vibrational spectroscopy, using a first-prin…