activity
20092014
most citedTwo-Dimensional Stimulated Resonance Raman Spectroscopy of Molecules with Broadband X-ray Pulses

73 citations · 150 across the 4 of their papers we have counts for

collaborators

6 papers

physics.chem-ph2014★ 35 cited

Time-, Frequency-, and Wavevector-Resolved X-Ray Diffraction from Single Molecules

Kochise Bennett, Jason D. Biggs, Yu Zhang +2

Using a quantum electrodynamic framework, we calculate the off-resonant scattering of a broad-band X-ray pulse from a sample initially prepared in an arbitrary superposition of ele…

physics.atom-ph2013★ 17 cited

Double-core Excitations in Formamide Can Be Probed by X-ray Double-quantum-coherence Spectroscopy

Yu Zhang, Daniel Healion, Jason D. Biggs +1

The attosecond, time-resolved X-ray double-quantum-coherence (XDQC) four wave mixing signals of formamide at the nitrogen and oxygen K-edges are simulated using restricted excitati…

physics.chem-ph2013★ 25 cited

Multidimensional X-Ray Spectroscopy of Valence and Core Excitations in Cysteine

Jason D. Biggs, Yu Zhang, Daniel Healion +1

Several nonlinear spectroscopy experiments which employ broadband x-ray pulses to probe the coupling between localized core and delocalized valence excitation are simulated for the…

physics.chem-ph2012★ 73 cited

Two-Dimensional Stimulated Resonance Raman Spectroscopy of Molecules with Broadband X-ray Pulses

Jason D. Biggs, Yu Zhang, Daniel Healion +1

Expressions for the two-dimensional Stimulated x-ray Raman Spectroscopy (2D-SXRS) signal obtained using attosecond x-ray pulses are derived. The 1D- and 2D-SXRS signals are calcula…

quant-ph2009

Calculations of Nonlinear Wave-Packet Interferometry Signals in the Pump-Probe Limit as Tests for Vibrational Control over Electronic Excitation Transfer

Jason D. Biggs, Jeffrey A. Cina

The preceding paper describes a strategy for externally influencing the course of short-time electronic excitation transfer (EET) in molecular dimers and observing the process by n…

quant-ph2009

Using Wave-Packet Interferometry to Monitor the External Vibrational Control of Electronic Excitation Transfer

Jason D. Biggs, Jeffrey A. Cina

We investigate the control of electronic energy transfer in molecular dimers through the preparation of specific vibrational coherences prior to electronic excitation, and its obse…