Carbonyl Vibrational Wave Packet Circulation in Mn${}_2$(CO)${}_{10}$ Driven by Ultrashort Polarized Laser Pulses

Mahmoud K. Abdel-Latif, Oliver Kühn

The excitation of the degenerate $E_1$ carbonyl stretching vibrations in dimanganese decacarbonyl is shown to trigger wave packet circulation in the subspace of these two modes. On…