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The critical role of the donor polymer in the stability of high-performance non-fullerene acceptor organic solar cells
Yiwen Wang, Alberto Privitera, Giacomo Londi +7
Driven by the rapid development of non-fullerene electron acceptors (NFAs), the power conversion efficiencies of organic solar cells (OSCs) have reached levels suitable for commerc…
Dielectric control of reverse intersystem crossing in thermally-activated delayed fluorescence emitters
Alexander J. Gillett, Anton Pershin, Raj Pandya +12
Thermally-activated delayed fluorescence (TADF) enables organic semiconductors with charge transfer (CT)-type excitons to convert dark triplet states into bright singlets via a rev…
Spontaneous exciton dissociation enables spin state interconversion in delayed fluorescence organic semiconductors
Alexander J. Gillett, Claire Tonnelé, Giacomo Londi +17
Engineering a low singlet-triplet energy gap (ΔEST) is necessary for efficient reverse intersystem crossing (rISC) in delayed fluorescence (DF) organic semiconductors, but results…
Analysis of external and internal disorder to understand band-like transport in n-type organic semiconductors
Marc-Antoine Stoeckel, Yoann Olivier, Marco Gobbi +18
Charge transport in organic semiconductors is notoriously extremely sensitive to the presence of disorder, both internal and external (i.e. related to the interactions with the die…
Structural and dynamic disorder, not ionic trapping, controls charge transport in highly doped conducting polymers
Ian E. Jacobs, Gabriele D'Avino, Vincent Lemaur +18
Doped organic semiconductors are critical to emerging device applications, including thermoelectrics, bioelectronics, and neuromorphic computing devices. It is commonly assumed tha…