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Quantifying Capacity Loss due to Solid-Electrolyte-Interphase Layer Formation on Silicon Negative Electrodes in Lithium-ion Batteries
Siva P. V. Nadimpalli, Vijay A. Sethuraman, Swapnil Dalavi +4
Charge lost per unit surface area of a silicon electrode due to the formation of solid-electrolyte-interphase (SEI) layer during initial lithiation was quantified, and the species…
Real-Time Stress Measurements in Lithium-ion Battery Negative-electrodes
Vijay A. Sethuraman, Nathan Van Winkle, Daniel P. Abraham +2
Real-time stress evolution in a graphite-based lithium-ion battery negative-electrode during electrolyte wetting and electrochemical cycling is measured through wafer-curvature met…
Analysis of Lithiation and Delithiation Kinetics in Silicon
Vijay A. Sethuraman, Venkat Srinivasan, John Newman
Analysis of lithiation and delithiation kinetics in pulse-laser-deposited crystalline thin-film silicon (Si) electrodes is presented. Data from open-circuit relaxation experiments…
Capacity Fade due to Side-reactions in Silicon Anodes in Lithium-ion Batteries
Vijay A. Sethuraman
It is shown that continuously occurring electrolyte-reduction reaction on freshly-exposed electrode surfaces during lithiation/delithiation cycles causes the lowering of cycling ef…