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Background-free measurement of exciton-exciton annihilation by two-quantum fluorescence-detected pump-probe spectroscopy
Ajay Jayachandran, Stefan Mueller, Christoph Lambert +1
We introduce two-quantum (2Q) fluorescence-detected pump-probe (F-PP) spectroscopy as a tool to probe ultrafast multiparticle interactions in many-body systems. We describe a pulse…
Probing plexciton dynamics with higher-order spectroscopy
Simon Büttner, Luca Nils Philipp, Julian Lüttig +5
Coupling molecular transition dipole moments to surface-plasmon polaritons (SPPs) results in the formation of new optical quasiparticles, i.e., plexcitons. Mixing the specific prop…
Separating orders of response in transient absorption and coherent multi-dimensional spectroscopy by intensity variation
Jacob J. Krich, Luisa Brenneis, Peter A. Rose +5
Interpretation of time-resolved spectroscopies such as transient absorption (TA) or two-dimensional (2D) spectroscopy often relies on the perturbative description of light-matter i…