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Femtosecond Laser Induced Coulomb Explosion Imaging of Aligned OCS Oligmers inside Helium Nanodroplets
James D. Pickering, Benjamin Shepperson, Lars Christiansen +1
Dimers and trimers of carbonyl sulfide (OCS) molecules embedded in helium nanodroplets are aligned by a linearly polarized 160 ps long moderately intense laser pulse and Coulomb ex…
Long-lasting field-free alignment of large molecules inside helium nanodroplets
Adam S. Chatterley, Constant Schouder, Lars Christiansen +3
Molecules with their axes sharply confined in space, available through laser-induced alignment methods, are essential for many current experiments, including ultrafast molecular im…
Molecular movie of ultrafast coherent rotational dynamics
Evangelos T. Karamatskos, Sebastian Raabe, Terry Mullins +10
Recording molecular movies on ultrafast timescales has been a longstanding goal for unravelling detailed information about molecular dynamics. We present the direct experimental re…
Hyperfine-Structure-Induced Depolarization of Impulsively Aligned Molecules
Esben F. Thomas, Anders A. Søndergaard, Benjamin Shepperson +2
A moderately intense fs laser pulse is used to create rotational wave packets in gas phase molecules. The ensuing time-dependent alignment, measured by Coulomb exp…
Switched Wave Packets with Spectrally Truncated Chirped Pulses
Adam Simon Chatterley, Evangelos Thomas Karamatskos, Constant Schouder +5
A new technique for obtaining switched wave packets using spectrally truncated chirped laser pulses is demonstrated experimentally and numerically by one-dimensional alignment of b…