10 citations · 14 across the 10 of their papers we have counts for
11 papers
Mutually phase-stable tunable attosecond soft X-ray attosecond pulses from a free-electron laser
River Robles, Kurtis Borne, Mathew Britton +16
We demonstrate the production of mutually phase-stable attosecond X-ray pulse pairs with tunable relative time delays and phases in a cascaded X-ray free-electron laser. We showcas…
Elucidating Norrish Type-I reactive pathways by ultrafast X-ray absorption spectroscopy
Martin Graßl, Pablo Unzueta, Andreas E. Hillers-Bendtsen +20
Norrish type I reactions selectively cleave carbon-carbon bonds directly adjacent to carbonyl groups. Despite their broad use in combination with aromatic carbonyls for additive ma…
Advanced Control of Electron Beams: Tailoring X-ray Production with Programmable Laser Shaping
Jack Hirschman, Randy Lemons, Hao Zhang +23
Leveraging the full scientific capabilities of next-generation high-repetition-rate free-electron lasers requires programmable control over electron-beam properties at their source…
Nonlinear reversal of photo-excitation on the attosecond time scale improves ultrafast x-ray diffraction images
Anatoli Ulmer, Phay J. Ho, Bruno Langbehn +28
The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectros…
Imaging valence electron rearrangement in a chemical reaction using hard X-ray scattering
Ian Gabalski, Alice Green, Philipp Lenzen +24
We have observed the signatures of valence electron rearrangement in photoexcited ammonia using ultrafast hard X-ray scattering. Time-resolved X-ray scattering is a powerful tool f…
Covariance Analysis of Impulsive Streaking
Jun Wang, Zhaoheng Guo, Erik Isele +4
We present a comprehensive framework of modeling covariance in angular streaking experiments. Within the impulsive streaking regime, the displacement of electron momentum distribut…
Attosecond Coherent Electron Motion in a Photoionized Aromatic Molecule
Taran Driver, Zhaoheng Guo, Erik Isele +50
In molecular systems, the ultrafast motion of electrons initiates the process of chemical change. Tracking this electronic motion across molecules requires coupling attosecond time…
"Beam `a la carte": laser heater shaping for attosecond pulses in a multiplexed x-ray free-electron laser
Siqi Li, Zhen Zhang, Shawn Alverson +19
Electron beam shaping allows the control of the temporal properties of x-ray free-electron laser pulses from femtosecond to attosecond timescales. Here we demonstrate the use of a…
Spectrotemporal shaping of attosecond x-ray pulses with a fresh-slice free-electron laser
River R. Robles, Kirk A. Larsen, David Cesar +14
We propose a scheme allowing coherent shaping, i.e., controlling both the amplitude and phase, of attosecond x-ray pulses at free-electron lasers. We show that by seeding an FEL wi…
Attosecond Delays in X-ray Molecular Ionization
Taran Driver, Miles Mountney, Jun Wang +34
The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the re…
Experimental Demonstration of Attosecond Pump-Probe Spectroscopy with an X-ray Free-Electron Laser
Zhaoheng Guo, Taran Driver, Sandra Beauvarlet +47
Pump-probe experiments with sub-femtosecond resolution are the key to understanding electronic dynamics in quantum systems. Here we demonstrate the generation and control of sub-fe…