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Photoinduced enhancement of chemical shift sensitivity to local vibrations
Ana Martínez Gutiérrez, Oliver Alexander, Pablo Estévez Alonso +26
The advent of novel free-electron laser sources enabling time-resolved x-ray photoelectron spectroscopy (tr-XPS) provides a unique opportunity to monitor local chemical environment…
Probing the structure of cyclic hydrocarbon molecules with X-ray-induced Coulomb explosion imaging
Kurtis D. Borne, Rebecca Boll, Thomas M. Baumann +27
Coulomb explosion imaging (CEI) is a powerful experimental technique that maps a molecule's geometric structure onto the momenta of ionic molecular fragments produced by rapid mult…
Unraveling real-time chemical shifts in the ultrafast regime
Daniel E. Rivas, Lorenzo Paoloni, Rebecca Boll +21
Traditional x-ray photoelectron spectroscopy (XPS) relies upon a direct mapping between the photoelectron binding energies and the local chemical environment, which is well-charact…
Unraveling the relaxation dynamics of Uracil: insights from time-resolved X-ray photoelectron spectroscopy
Davide Faccialà, Matteo Bonanomi, Bruno Nunes Cabral Tenorio +26
We report a study of the electronic and nuclear relaxation dynamics of the photoexcited RNA base uracil in the gas phase, using time-resolved core level photoelectron spectroscopy…
Controlled molecule injector for cold, dense, and pure molecular beams at the European x-ray free-electron laser
Lanhai He, Melby Johny, Thomas Kierspel +27
A permanently available molecular-beam injection setup for controlled molecules (COMO) was installed and commissioned at the small quantum systems (SQS) instrument at the European…