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Dominant spin-spin relaxation mechanism at clock transition of the complex at different concentrations
Xiao Chen, Haechan Park, Silas Hoffman +2
Spin decoherence poses a significant challenge in molecular magnets, with the nuclear spin bath serving as a prominent source. Intriguingly, spin qubits at the clock transition exh…
Floquet Engineering Clock Transitions in Magnetic Molecules
Andrew Cupo, Shuanglong Liu, Silas Hoffman +2
We theoretically study Floquet engineering of magnetic molecules via a time-periodic magnetic field that couples to the emergent total electronic spin of the metal center. By focus…
Simulating decoherence of two coupled spins using the generalized cluster correlation expansion
Xiao Chen, Silas Hoffman, James N. Fry +1
We simulate the coherence of two coupled electron spins interacting with a bath of nuclei using the generalized cluster correlation expansion (gCCE) method. An exchange interaction…