8 papers
Photoinduced enhancement of chemical shift sensitivity to local vibrations
Ana MartÃnez Gutiérrez, Oliver Alexander, Pablo Estévez Alonso +26
The advent of novel free-electron laser sources enabling time-resolved x-ray photoelectron spectroscopy (tr-XPS) provides a unique opportunity to monitor local chemical environment…
Attosecond soft X-ray pulses generated by chirp-dispersed manipulation in an XFEL reveal nonlinear core-electron dynamics in neon
Lars Funke, Markus Ilchen, Svitozar Serkez +59
Free-electron lasers have demonstrated their capability of generating intense attosecond X-ray pulses, which are the key to studying electron dynamics at their natural time scale a…
Probing the structure of cyclic hydrocarbon molecules with X-ray-induced Coulomb explosion imaging
Kurtis D. Borne, Rebecca Boll, Thomas M. Baumann +27
Coulomb explosion imaging (CEI) is a powerful experimental technique that maps a molecule's geometric structure onto the momenta of ionic molecular fragments produced by rapid mult…
Unraveling real-time chemical shifts in the ultrafast regime
Daniel E. Rivas, Lorenzo Paoloni, Rebecca Boll +21
Traditional x-ray photoelectron spectroscopy (XPS) relies upon a direct mapping between the photoelectron binding energies and the local chemical environment, which is well-charact…
Dichroic Electron Emission Patterns from Oriented Helium Ions
Niclas Wieland, Klaus Bartschat, Filippa Dudda +17
We report a joint experimental and theoretical study using a combination of polarization-controlled free-electron-laser (FEL) and near-infra\-red (NIR) pulses in a synchronized two…
Probing the Linewidth of the 12.4-keV Solid-State Sc Isomeric Resonance
Peifan Liu, Miriam Gerharz, Berit Marx-Glowna +37
The Sc nuclear transition from the ground to the isomeric state at 12.389~keV, with a lifetime of 0.46~s, exhibits an extraordinarily narrow natural width of 1.4~feV and a q…