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Nonlinear spectroscopy with entangled photons; manipulating quantum pathways of matter
O. Roslyak C. A. Marx, S. Mukamel
Optical signals obtained by the material response to classical laser fields are given by nonlinear response functions which can be expressed by sums over various quantum pathways o…
Theory of enhanced dynamical photo-thermal bi-stability effects in cuprous oxide/organic hybrid heterostructure
Oleksiy Roslyak, Joseph L. Birman
We theoretically demonstrate the formation of multiple bi-stability regions in the temperature pattern on the interface between a cuprous oxide quantum well and DCM2:CA:PS organic…
Polaritons in cuprous oxide perturbed by LA-phonons
Oleksiy Roslyak, Joseph L. Birman
We present a comparative analysis of a 'conventional' phonoriton (coherent superposition of exciton-photon-phonon) and a polariton (coherent exciton-photon superposition) 'weakly'…
Theory of enhanced second-harmonic generation by the quadrupole-dipole hybrid exciton
Oleksiy Roslyak, Joseph L. Birman
We report calculated substantial enhancement of the second harmonic generation (SHG) in cuprous oxide crystals resonantly hybridized with an appropriate organic material (DCM2:CA:P…
Hybridized quadrupole-dipole exciton effects in - Organic Heterostructure
Oleksiy Roslyak, Joseph L. Birman
In the present work we discuss resonant hybridization of the quadrupole Wannier-Mott exciton (WE) in a quantum well with the Frenkel (FE) dipole exciton in an adjacent…