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Selectivity in tip-induced skeletal editing via heteroatom substitution
Shantanu Mishra, Rasmus Svensson, Valentina Malave +5
Skeletal editing enables precise structural modifications of molecules at late stages of a synthetic sequence, with applications in drug discovery and materials science. We recentl…
On-surface synthesis and aromaticity of large cyclocarbons
Lisanne Sellies, Marco Vitek, Yueze Gao +12
Molecular rings of N carbon atoms, that is, cyclo[N]carbons, or C, can be formed by tip-induced chemistry [1-7]. Because of their monocyclic geometry, cyclocarbons are fundamen…
A molecule with half-Möbius topology
Igor Roncevic, Fabian Paschke, Yueze Gao +10
Stereoisomers of CCl exhibiting helical orbitals around a ring of carbon atoms were synthesized by atom manipulation on NaCl surfaces. We resolved the enantiomeric geome…
Skeletal editing by tip-induced chemistry
Shantanu Mishra, Valentina Malave, Rasmus Svensson +4
Skeletal editing of cyclic molecules has garnered considerable attention in the context of drug discovery and green chemistry, with notable examples in solution-phase synthesis. He…
Synthesis and characterization of a -extended Clar's goblet
Shantanu Mishra, Manuel Vilas-Varela, Igor RonÄeviÄ +4
Concealed non-Kekulé polybenzenoid hydrocarbons have no sublattice imbalance yet cannot be assigned a classical Kekulé structure, leading to an open-shell ground state with poten…
A Route Toward the On-Surface Synthesis of Organic Ferromagnetic Quantum Spin Chains
Fabian Paschke, Ricardo Ortiz, Shantanu Mishra +5
Engineering sublattice imbalance is an intuitive way to induce high-spin ground states in bipartite polycyclic conjugated hydrocarbons (PCHs). Such high-spin molecules can be emplo…