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Quantum Vibronic Dynamics Shape Catalytically Relevant Au-Ligand Interfaces in Atomically Precise Gold Nanoclusters
Mengyuan Cui, Tianrui Chen, Junhua Zhou +6
Atomically precise gold nanoclusters are versatile for photocatalysis and energy conversion because their electronic structure stems from strong metal-ligand interactions. However,…
Environmental Control Extends Beyond Quantum Dephasing in Exciton Energy Transfer
Junhua Zhou, Tianrui Chen, Dehao Yuan +8
Excitation-energy transfer underpins the conversion of light into usable energy in photosynthetic organisms and serves as a paradigm for evolutionary optimized transport in open qu…
Conical Intersections Enable Ultrafast Molecular Spin Control in a Chromium Complex
Zihui Liu, Junhua Zhou, Tianrui Chen +8
Molecular spintronics seeks to control spin states in single molecules for ultrafast switching and efficient information processing. Transition metal complexes are promising candid…
Excitonic Energy Transfer in Red Algal Photosystem I Reveals an Evolutionary Bridge between Cyanobacteria and Plants
Mengyuan Cui, Zihui Liu, Miriam Izzo +9
Photosystem I converts light into chemical energy with near-unity quantum efficiency,yet its energy-transfer and charge-separation mechanisms remain debated. Evolution has diversif…
Diverse Transient Chiral Dynamics in Evolutionary distinct Photosynthetic Reaction Centers
Yonglei Yang, Zihui Liu, Fulu Zheng +4
The evolution of photosynthetic reaction centers (RCs) from anoxygenic bacteria to oxygenic cyanobacteria and plants reflects their structural and functional adaptation to environm…
Unraveling Quantum Coherences Mediating Primary Charge Transfer Processes in Photosystem II Reaction Center
Ajay Jha, Pan-Pan Zhang, Vandana Tiwari +4
Photosystem II (PSII) reaction center is a unique protein-chromophore complex that is capable of efficiently separating electronic charges across the membrane after photoexcitation…