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physics.optics2008
A general theory of inhomogeneous broadening for nonlinear susceptibilities: the second hyperpolarizability
Robert J. Kruhlak, Mark G. Kuzyk
A general theory of inhomogeneous broadening is rarely applied to nonlinear spectroscopy in lieu of either a simple Lorentzian or Gaussian model. In this work, we generalize all th…
physics.optics2008
A general theory of inhomogeneous broadening for nonlinear susceptibilities: polarizability and hyperpolarizability
Robert J. Kruhlak, Mark G. Kuzyk
While nonlinear optical spectroscopy is becoming more commonly used to study the excited states of nonlinear-optical systems, a general theory of inhomogeneous broadening is rarely…