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72 papers
Quantum Efficiency of Single Dibenzoterrylene Molecules in para-Dichlorobenzene at Cryogenic Temperatures
Mohammad Musavinezhad, Dominik Rattenbacher, Alexey Shkarin +4
We measure the quantum efficiency (QE) of individual dibenzoterrylene (DBT) molecules embedded in para-dichlorobenzene at cryogenic temperatures. To achieve this, we apply two dist…
Spectral splitting of a stimulated Raman transition in a single molecule
Johannes Zirkelbach, Burak Gurlek, Masoud Mirzaei +4
The small cross section of Raman scattering poses a great challenge for its direct study at the single-molecule level. By exploiting the high Franck-Condon factor of a common-mode…
On-chip interference of scattering from two individual molecules in plastic
Dominik Rattenbacher, Alexey Shkarin, Jan Renger +3
Integrated photonic circuits offer a promising route for studying coherent cooperative effects of a controlled collection of quantum emitters. However, spectral inhomogeneities, de…
A robust tip-less positioning device for near-field investigations: Press and Roll Scan (PROscan)
Hsuan-Wei Liu, Michael A. Becker, Korenobu Matsuzaki +3
Scanning probe microscopes scan and manipulate a sharp tip in the immediate vicinity of a sample surface. The limited bandwidth of the feedback mechanism used for stabilizing the s…
High-resolution vibronic spectroscopy of a single molecule embedded in a crystal
Johannes Zirkelbach, Masoud Mirzaei, Irena Deperasinska +6
Vibrational levels of the electronic ground states in dye molecules have not been previously explored at high resolution in solid matrices. We present new spectroscopic measurement…
Single-molecule vacuum Rabi splitting: four-wave mixing and optical switching at the single-photon level
André Pscherer, Manuel Meierhofer, Daqing Wang +5
A single quantum emitter can possess a very strong intrinsic nonlinearity, but its overall promise for nonlinear effects is hampered by the challenge of efficient coupling to incid…