activity
20212025
most citedMolecular Structure Optimization based on Electrons-Nuclei Quantum Dynamics Computation

12 citations · 25 across the 7 of their papers we have counts for

collaborators

7 papers

physics.chem-ph2025★ 1 cited

Enhancing Accuracy of Quantum-Selected Configuration Interaction Calculations using Multireference Perturbation Theory: Application to Aromatic Molecules

Soichi Shirai, Shih-Yen Tseng, Hokuto Iwakiri +3

Quantum-selected configuration interaction (QSCI) is a novel quantum-classical hybrid algorithm for quantum chemistry calculations. This method identifies electron configurations h…

physics.chem-ph2024

Theoretical analysis of chemical reactions using a variational quantum eigensolver method without specifying molecular charge

Soichi Shirai, Takahiro Horiba, Hirotoshi Hirai

Quantum chemical calculations have attracted much attention as a practical application of quantum computing. Quantum computers can prepare superpositions of electronic states with…

quant-ph2023

Construction of Antisymmetric Variational Quantum States with Real-Space Representation

Takahiro Horiba, Soichi Shirai, Hirotoshi Hirai

Electronic state calculations using quantum computers are mostly based on second quantization, which is suitable for qubit representation. Another way to describe electronic states…

physics.chem-ph2023

Computational analysis of chemical reactions using a variational quantum eigensolver algorithm without specifying spin multiplicity

Soichi Shirai, Hokuto Iwakiri, Keita Kanno +4

The analysis of a chemical reaction along the ground state potential energy surface in conjunction with an unknown spin state is challenging because electronic states must be separ…

physics.chem-ph2021★ 8 cited

Calculation of core-excited and core-ionized states using variational quantum deflation method and applications to photocatalyst modelling

Soichi Shirai, Takahiro Horiba, Hirotoshi Hirai

The possibility of performing quantum chemical calculations using quantum computers has attracted much interest. In this regard, variational quantum deflation (VQD) is a quantum-cl…

quant-ph2021★ 4 cited

Missing Rung Problem in Vibrational Ladder Climbing

Takahiro Horiba, Soichi Shirai, Hirotoshi Hirai

We observed vanishing of the transition dipole moment, interrupting vibrational ladder climbing (VLC) in molecular systems. We clarified the mechanism of this phenomenon and presen…