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physics.optics2022
Accelerated Molecular Vibrational Decay and Suppressed Electronic Nonlinearities in Plasmonic Cavities through Coherent Raman Scattering
Lukas A. Jakob, William M. Deacon, Rakesh Arul +3
Molecular vibrations and their dynamics are of outstanding importance for electronic and thermal transport in nanoscale devices as well as for molecular catalysis. The vibrational…
physics.optics2022★ 55 cited
Giant optomechanical spring effect in plasmonic nano- and picocavities probed by surface-enhanced Raman scattering
Lukas A. Jakob, William M. Deacon, Yuan Zhang +8
Molecular vibrations couple to visible light only weakly, have small mutual interactions, and hence are often ignored for non-linear optics. Here we show the extreme confinement pr…