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Coherent Control of Ion-Photoelectron Dynamics through Rabi Oscillations: An ab initio study
Bo-Ren Shen, Yi-Jia Mao, Zhao-Han Zhang +4
We present first-principles numerical simulations of photoionization in neon induced by bichromatic extreme ultraviolet pulses with frequencies and , specially chosen to ma…
Time-dependent Hole States in Multiconfigurational Time-Dependent Hartree-Fock Approaches: Applications in Photoionization of Water Molecule
Zhao-Han Zhang, Yang Li, Himadri Pathak +3
By simulating the real-time multielectron wavefunction with the multi-configurational time-dependent Hartree-Fock (MCTDHF) approach, we conduct an \textit{ab initio} study of the s…
Time-dependent Hole States in Multiconfigurational Time-Dependent Hartree-Fock Approaches: A Time-Domain Generalization of Extended Koopmans' Theorem
Zhao-Han Zhang, Yang Li, Himadri Pathak +3
We introduce a framework for resolving electron-hole dynamics within wavefunction-based multiconfigurational time-dependent Hartree-Fock (MCTDHF) theory. Central to this framework…
Ultrafast Two-electron Orbital Swap in Li Initiated by Attosecond pulses
Hui Jiang, Zhao-Han Zhang, Yang Li +2
A universal mechanism of ultrafast two-electron orbital swap is discovered through two-photon sequential double ionization of Li. After a electron in Li is ionized by absorbin…