activity
20202026
most citedFunctionalizing Aromatic Compounds with Optical Cycling Centers

49 citations · 73 across the 10 of their papers we have counts for

collaborators

10 papers

quant-ph2026

Yttrium ion as a platform for quantum information processing

Christopher N. Gilbreth, Dmytro Filin, Marianna S. Safronova +2

Engineering large-scale quantum computers which simultaneously provide high-fidelity quantum operations, low memory errors, low crosstalk, and reasonable resource usage remains an…

quant-ph2026

A Surface-Scaffolded Molecular Qubit

Tian-Xing Zheng, M. Iqbal Bakti Utama, Xingyu Gao +24

Fluorescent spin qubits are central building blocks of quantum technologies. Placing these qubits at surfaces maximizes coupling to nearby spins and fields, enabling nanoscale sens…

physics.chem-ph2025

Unraveling vibronic interactions in molecules functionalized with optical cycling centers

Pawel Wojcik, Haowen Zhou, Taras Khvorost +7

We report detailed characterization of the vibronic interactions between the first two electronically excited states, A and B, in SrOPh (Ph = phenyl, -C6H5) and its deuterated coun…

physics.atom-ph2025★ 2 cited

Vibronic coupling limits the use of high-lying electronic states in complex molecules for laser cooling

Haowen Zhou, Pawel Wojcik, Guo-Zhu Zhu +7

Laser cooling of large, complex molecules is a long-standing goal, instrumental for enabling new quantum technology and precision measurements. A primary consideration for the feas…

physics.chem-ph2024

Bottom-up approach to scalable growth of molecules capable of optical cycling

Guanming Lao, Taras Khvorost, Antonio Macias +10

Gas-phase molecules capable of repeatable, narrow-band spontaneous photon scattering are prized for direct laser cooling and quantum state detection. Recently, large molecules inco…

physics.chem-ph2023

Extending the large molecule limit: The role of Fermi resonance in developing a quantum functional group

Guo-Zhu Zhu, Guanming Lao, Claire E. Dickerson +4

Polyatomic molecules equipped with optical cycling centers (OCCs), enabling continuous photon scattering during optical excitation, are exciting candidates for advancing quantum in…

physics.atom-ph2022★ 14 cited

Laser spectroscopy of aromatic molecules with optical cycling centers: strontium (I) phenoxides

Guanming Lao, Guo-Zhu Zhu, Claire E. Dickerson +5

We report the production and spectroscopic characterization of strontium (I) phenoxide (, or SrOPh) and variants featuring electron-withdrawing groups…

physics.atom-ph2022★ 49 cited

Functionalizing Aromatic Compounds with Optical Cycling Centers

Guo-Zhu Zhu, Debayan Mitra, Benjamin L. Augenbraun +9

Molecular design principles provide guidelines for augmenting a molecule with a smaller group of atoms to realize a desired property or function. We demonstrate that these concepts…

physics.chem-ph2021★ 8 cited

High-resolution laser-induced fluorescence spectroscopy of SiO and SiO in a cryogenic buffer-gas cell

Guo-Zhu Zhu, Guanming Lao, Clayton Ho +2

The electronic, laser-induced fluorescence spectrum of the transition in SiO and SiO has been recorded in a cryogenic…

physics.optics2020

Interaction between vortex beams and diatomic molecules with rotation

Guanming Lao

The interaction between vortex beam (VB) and molecule has drawn much attention in recent years, but the lack of theoretical method somehow limits its further analysis, especially w…