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physics.optics2011★ 12 cited
A quantum mechanical model of the upper bounds of the cascading contribution to the second hyperpolarizability
Nathan J. Dawson, Benjamin R. Anderson, Jennifer L. Schei +1
Microscopic cascading of second-order nonlinearities between two molecules has been proposed to yield an enhanced third-order molecular nonlinear-optical response. In this contribu…
physics.optics2011★ 13 cited
A classical model of the upper bounds of the cascading contribution to the second hyperpolarizability
Nathan J. Dawson, Benjamin R. Anderson, Jennifer L. Schei +1
We investigate whether microscopic cascading of second-order nonlinearities of two molecules in the side-by-side configuration can lead to a third-order molecular nonlinear-optical…