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Laser spectroscopy of aromatic molecules with optical cycling centers: strontium (I) phenoxides
Guanming Lao, Guo-Zhu Zhu, Claire E. Dickerson +5
We report the production and spectroscopic characterization of strontium (I) phenoxide (, or SrOPh) and variants featuring electron-withdrawing groups…
Bethe Salpeter Equation Spectra for Very Large Systems
Nadine Bradbury, Minh Nguyen, Justin R Caram +1
We present a highly efficient method for the extraction of optical properties of very large molecules via the Bethe-Salpeter equation. The crutch of this approach is the calculatio…
Pathway Towards Optical Cycling and Laser Cooling of Functionalized Arenes
Debayan Mitra, Zack D. Lasner, Guo-Zhu Zhu +8
Rapid and repeated photon cycling has enabled precision metrology and the development of quantum information systems using a variety of atoms and simple molecules. Extending optica…
Functionalizing Aromatic Compounds with Optical Cycling Centers
Guo-Zhu Zhu, Debayan Mitra, Benjamin L. Augenbraun +9
Molecular design principles provide guidelines for augmenting a molecule with a smaller group of atoms to realize a desired property or function. We demonstrate that these concepts…