64 citations · 186 across the 10 of their papers we have counts for
10 papers
A digitally controlled silicon quantum processing unit
Members of the HRL Quantum Team, Collaborators, : +255
Commercially-relevant quantum computers will require large numbers of high-performing qubits that can be manufactured, integrated, and controlled at scale. Silicon exchange-only (E…
Extending the large molecule limit: The role of Fermi resonance in developing a quantum functional group
Guo-Zhu Zhu, Guanming Lao, Claire E. Dickerson +4
Polyatomic molecules equipped with optical cycling centers (OCCs), enabling continuous photon scattering during optical excitation, are exciting candidates for advancing quantum in…
Single molecule superradiance for optical cycling
Claire E. Dickerson, Anastassia N. Alexandrova, Prineha Narang +1
Herein, we show that single molecules containing multiple optical cycling centers (CaO moieties) can exhibit superradiant phenomena. We demonstrate the accuracy of the Frenkel exci…
Probing the limits of optical cycling in a predissociative diatomic molecule
Qi Sun, Claire E. Dickerson, Jinyu Dai +6
Molecular predissociation is the spontaneous, nonradiative bond breaking process that can occur upon excitation. In the context of laser cooling, predissociation is an unwanted con…
Laser spectroscopy of aromatic molecules with optical cycling centers: strontium (I) phenoxides
Guanming Lao, Guo-Zhu Zhu, Claire E. Dickerson +5
We report the production and spectroscopic characterization of strontium (I) phenoxide (, or SrOPh) and variants featuring electron-withdrawing groups…
Fully saturated hydrocarbons as hosts of optical cycling centers
Claire E. Dickerson, Cecilia Chang, Han Guo +1
Designing closed, laser-induced optical cycling transitions in trapped atoms or molecules is useful for quantum information processing, precision measurement, and quantum sensing.…
Pathway Towards Optical Cycling and Laser Cooling of Functionalized Arenes
Debayan Mitra, Zack D. Lasner, Guo-Zhu Zhu +8
Rapid and repeated photon cycling has enabled precision metrology and the development of quantum information systems using a variety of atoms and simple molecules. Extending optica…
Functionalizing Aromatic Compounds with Optical Cycling Centers
Guo-Zhu Zhu, Debayan Mitra, Benjamin L. Augenbraun +9
Molecular design principles provide guidelines for augmenting a molecule with a smaller group of atoms to realize a desired property or function. We demonstrate that these concepts…
Analog quantum simulation of chemical dynamics
Ryan J. MacDonell, Claire E. Dickerson, Clare J. T. Birch +5
Ultrafast chemical reactions are difficult to simulate because they involve entangled, many-body wavefunctions whose computational complexity grows rapidly with molecular size. In…
Franck-Condon tuning of optical cycling centers by organic functionalization
Claire E. Dickerson, Han Guo, Ashley J. Shin +4
Laser induced electronic excitations that spontaneously emit photons and decay directly to the initial ground state ("optical cycling transitions") are used in quantum information…