activity
20212026
most citedImproved Spin-State Energy Differences of Fe(II) molecular and crystalline complexes via the Hubbard U-corrected Density

8 citations · 9 across the 9 of their papers we have counts for

collaborators

10 papers

quant-ph2026

Triangulene-based diradicals as a blueprint for molecular quantum platforms with optical addressability and long spin coherence times

Arup Sarkar, Cathal Hogan, Conor Ryan +2

The identification of molecules that combine long spin coherence times and efficient spin-optical interfaces, ideally at room temperature, is pivotal towards the development of mol…

cond-mat.mtrl-sci2026

Raman relaxation in Yb(III) molecular qubits: non-trivial correlations between spin-phonon coupling and molecular structure

Giacomo Sansone, Lorenzo A. Mariano, Stefano Carretta +2

The coordination complexes of Yb(III) exhibit some of the longest spin coherence times among 4f compounds, making them a promising platform for molecular quantum technologies. Whil…

cond-mat.mtrl-sci20261 cited

Efficient training of generative models from multireference simulations and its application to the design of Dy complexes with large magnetic anisotropy

Zahra Khatibi, Lorenzo A. Mariano, Lion Frangoulis +1

Generative machine learning models can potentially provide direct access to novel and relevant portions of the full chemical space, overcoming the cost of systematic sampling. Howe…

cond-mat.mtrl-sci2025

Generating new coordination compounds via multireference simulations, genetic algorithms and machine learning: the case of Co(II) molecular magnets

Lion Frangoulis, Zahra Khatibi, Lorenzo A. Mariano +1

The design of coordination compounds with target properties often requires years of continuous feedback loop between theory, simulations and experiments. In the case of magnetic mo…

cond-mat.mtrl-sci2024

The Mechanism of Spin-Phonon Relaxation in Endohedral Metallofullene Single Molecule Magnets

Tanu Sharma, Rupesh Kumar Tiwari, Sourav Dey +3

This study presents the first-ever investigation of spin-phonon coupling mechanisms in fullerene-based single-molecule magnets (SMMs) using ab initio CASSCF combined with DFT calcu…

physics.chem-ph2024

Charting new regions of Cobalt's chemical space with maximally large magnetic anisotropy: A computational high-throughput study

Lorenzo A. Mariano, Vu Ha Anh Nguyen, Valerio Briganti +1

Magnetic anisotropy slows down magnetic relaxation and plays a prominent role in the design of permanent magnets. Coordination compounds of Co(II) in particular exhibit large magne…