most citedChemical tuning of spin clock transitions in molecular monomers based on nuclear spin-free Ni(II)

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quant-ph2021★ 34 cited

Chemical tuning of spin clock transitions in molecular monomers based on nuclear spin-free Ni(II)

Marcos Rubín-Osanz, François Lambert, Feng Shao +8

We report the existence of a sizeable quantum tunnelling splitting between the two lowest electronic spin levels of mononuclear Ni complexes. The level anti-crossing, or magnetic c…