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physics.chem-ph2021★ 16 cited
Distribution of first-reaction times with target regions on boundaries of shell-like domains
Denis S. Grebenkov, Ralf Metzler, Gleb Oshanin
We study the probability density function (PDF) of the first-reaction times between a diffusive ligand and a membrane-bound, immobile imperfect target region in a restricted "onion…
physics.chem-ph2019★ 129 cited
Strong defocusing of molecular reaction times results from an interplay of geometry and reaction control
Denis S. Grebenkov, Ralf Metzler, Gleb Oshanin
Text-book concepts of diffusion- versus kinetic-control are well-defined for reaction-kinetics involving macroscopic concentrations of diffusive reactants that are adequately descr…