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20172026
most citedIs the Trotterized UCCSD Ansatz chemically well-defined?

168 citations · 380 across the 29 of their papers we have counts for

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physics.chem-ph2025

Computing Exchange Coupling constants in Transition metal complexes with Tensor Product Selected Configuration Interaction

Arnab Bachhar, Nicholas J. Mayhall

Transition metal complexes present significant challenges for electronic structure theory due to strong electron correlation arising from partially filled -orbitals. We compare…

physics.chem-ph2024

Restricted Open-shell cluster Mean-Field theory for Strongly Correlated Systems

Arnab Bachhar, Nicholas J. Mayhall

The cluster-based Mean Field method (cMF) and it's second order perturbative correction[1], was introduced by Jiménez-Hoyos and Scuseria to reduce the cost of modeling strongly cor…

physics.chem-ph2024

Accurate and Interpretable Representation of Correlated Electronic Structure via Tensor Product Selected CI

Nicole M. Braunscheidel, Arnab Bachhar, Nicholas J. Mayhall

The task of computing wavefunctions that are accurate, yet simple enough mathematical objects to use for reasoning has long been a challenge in quantum chemistry. The difficulty in…

physics.chem-ph2023

Generalization of the tensor product selected CI method for molecular excited states

Nicole M. Braunscheidel, Vibin Abraham, Nicholas J. Mayhall

In a recent paper [JCTC, 2020, 16, 6098], we introduced a new approach for accurately approximating full CI ground states in large electronic active-spaces, called Tensor Product S…

physics.chem-ph2022

New Local Explorations of the Unitary Coupled Cluster Energy Landscape

Harper R. Grimsley, Nicholas J. Mayhall

The recent quantum information boom has effected a resurgence of interest in unitary coupled cluster (UCC) theory. Our group's interest in local energy landscapes of unitary ansätz…

physics.chem-ph2022

Coupled electron pair-type approximations for tensor product state wavefunctions

Vibin Abraham, Nicholas J. Mayhall

Size extensivity, defined as the correct scaling of energy with system size, is a desirable property for any many-body method. Traditional CI methods are not size extensive hence t…