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physics.optics2022★ 2 cited
Controlling rotationally-resolved two-dimensional infrared spectra with polarization
Grzegorz Kowzan, Thomas K. Allison
Recent advancements in infrared frequency combs will enable recording of coherent two-dimensional infrared spectra of gas-phase molecules with rotational resolution (RR2DIR). We de…
physics.optics2022★ 2 cited
Theory of rotationally resolved two-dimensional infrared spectroscopy including polarization dependence and rotational coherence dynamics
Grzegorz Kowzan, Thomas K. Allison
Two-dimensional infrared (2DIR) spectroscopy is widely used to study molecular dynamics but it is typically restricted to solid and liquid phase samples and modest spectral resolut…