6 papers
Enhancing Spin Coherence in Optically Addressable Molecular Qubits through Host-Matrix Control
S. L. Bayliss, P. Deb, D. W. Laorenza +4
Optically addressable spins are a promising platform for quantum information science due to their combination of a long-lived qubit with a spin-optical interface for external qubit…
Optically addressable molecular spins for quantum information processing
S. L. Bayliss, D. W. Laorenza, P. J. Mintun +3
Spin-bearing molecules are promising building blocks for quantum technologies as they can be chemically tuned, assembled into scalable arrays, and readily incorporated into diverse…
Purcell enhancement of a single silicon carbide color center with coherent spin control
A. L. Crook, C. P. Anderson, K. C. Miao +9
Silicon carbide has recently been developed as a platform for optically addressable spin defects. In particular, the neutral divacancy in the 4H polytype displays an optically addr…
Spin fine-structure reveals bi-exciton geometry in an organic semiconductor
K. M. Yunusova, S. L. Bayliss, T. Chanelière +4
In organic semiconductors, bi-excitons are key intermediates in carrier-multiplication and exciton annihilation. Their local geometry governs their electronic properties and yet ha…
Electrically driven optical interferometry with spins in silicon carbide
Kevin C. Miao, Alexandre Bourassa, Christopher P. Anderson +11
Interfacing solid-state defect electron spins to other quantum systems is an ongoing challenge. The ground-state spin's weak coupling to its environment bestows excellent coherence…
Site-selective measurement of coupled spin pairs in an organic semiconductor
Sam L. Bayliss, Leah R. Weiss, Anatol Mitioglu +14
From organic electronics to biological systems, understanding the role of intermolecular interactions between spin pairs is a key challenge. Here we show how such pairs can be sele…