360 citations · 989 across the 12 of their papers we have counts for
14 papers
Optical Detection of Coherent Nuclear Spin Control in a Molecular System at Room Temperature
Eoin O. Irving, Ziqiu Huang, Max Attwood +2
Molecular systems with optically addressable electron spins are emerging as versatile quantum sensing platforms, offering tunable qubit properties and molecular-scale spatial contr…
Understanding the spin coherence of molecular photoexcited triplet states from first principles
Ecaterina Păunică, Sam L. Bayliss
Optically readable molecular spins are attractive as quantum sensors due to their nanoscale modularity, synthetic tunability, and scope for sensitive readout. In particular, photoe…
Host-guest Crystal Engineering Tailors the Room Temperature Spin Dynamics in Molecular Quantum Devices
Ziqiu Huang, Angus Cowley-Semple, Irena Nevjestic +5
Molecular materials that enable coherent control over an electron's spin state at room temperature are promising candidates for quantum technologies, including quantum sensors and…
Room temperature optical control of spin states in organic diradicals
Rituparno Chowdhury, Alistair Inglis, Lucy E. Walker +13
We report a family of luminescent alternant diradicals which, at room temperature, support a ground-state spin-triplet, near-unity photoluminescence quantum yields, and optical spi…
Chemically Tuning Room Temperature Pulsed Optically Detected Magnetic Resonance
Sarah K. Mann, Angus Cowley-Semple, Emma Bryan +4
Optical detection of magnetic resonance enables spin-based quantum sensing with high spatial resolution and sensitivity-even at room temperature-as exemplified by solid-state defec…
Room-temperature optically detected coherent control of molecular spins
Adrian Mena, Sarah K. Mann, Angus Cowley-Semple +5
Benefiting from both molecular tunability and versatile methods for deployment, optically interfaced molecular spins are a promising platform for quantum technologies such as sensi…
Enhancing Spin Coherence in Optically Addressable Molecular Qubits through Host-Matrix Control
S. L. Bayliss, P. Deb, D. W. Laorenza +4
Optically addressable spins are a promising platform for quantum information science due to their combination of a long-lived qubit with a spin-optical interface for external qubit…
Optically addressable molecular spins for quantum information processing
S. L. Bayliss, D. W. Laorenza, P. J. Mintun +3
Spin-bearing molecules are promising building blocks for quantum technologies as they can be chemically tuned, assembled into scalable arrays, and readily incorporated into diverse…
Purcell enhancement of a single silicon carbide color center with coherent spin control
A. L. Crook, C. P. Anderson, K. C. Miao +9
Silicon carbide has recently been developed as a platform for optically addressable spin defects. In particular, the neutral divacancy in the 4H polytype displays an optically addr…
Spin fine-structure reveals bi-exciton geometry in an organic semiconductor
K. M. Yunusova, S. L. Bayliss, T. Chanelière +4
In organic semiconductors, bi-excitons are key intermediates in carrier-multiplication and exciton annihilation. Their local geometry governs their electronic properties and yet ha…
Electrically driven optical interferometry with spins in silicon carbide
Kevin C. Miao, Alexandre Bourassa, Christopher P. Anderson +11
Interfacing solid-state defect electron spins to other quantum systems is an ongoing challenge. The ground-state spin's weak coupling to its environment bestows excellent coherence…
Site-selective measurement of coupled spin pairs in an organic semiconductor
Sam L. Bayliss, Leah R. Weiss, Anatol Mitioglu +14
From organic electronics to biological systems, understanding the role of intermolecular interactions between spin pairs is a key challenge. Here we show how such pairs can be sele…
Room temperature magneto-optic effect in silicon light-emitting diodes
F. Chiodi, S. L. Bayliss, L. Barast +4
In weakly spin-orbit coupled materials, the spin-selective nature of recombination can give rise to large magnetic-field effects, for example on electro-luminescence from molecular…
Ultrafast Triplet Pair Formation and Subsequent Thermally Activated Dissociation Control Efficient Endothermic Singlet Exciton Fission
Hannah L. Stern, Alexandre Cheminal, Shane R. Yost +12
Singlet exciton fission (SF), the conversion of one spin-singlet exciton (S1) into two spin-triplet excitons (T1), could provide a means to overcome the Shockley-Queisser limit in…