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high harmonic generation 1molecular alignment 1orbital angular momentum 1strong-field physics 1time-dependent density functional theory 1

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physics.chem-ph2026

Macroscopic Spin-Orbit Interaction through Strong-Field Pumping of Inhomogeneously Aligned Molecular Ensemble

Uriel Zanzuri, Sharly Fleischer, Tamar Seideman +3

The paper investigates how a helical bi‑chromatic strong‑field pump interacting with a radially aligned molecular ensemble generates high‑harmonic radiation that carries orbital an…