Spin-forbidden excitations in the magneto-optical spectra of CrI${}_3$ tuned by covalency

Connor A. Occhialini, Luca Nessi, Luiz G. P. Martins +10

Spin-forbidden ($\hat{I}”S\ne 0$) multiplet excitations and their coupling to magnetic properties are of increasing importance for magneto-optical studies of correlated materials. None…