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From the 1 of 7 linked papers with an AI index.

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7 papers

physics.chem-ph2026

Solid-State NMR Dipolar Recoupling in Presence of Large Chemical Shielding Anisotropies by Quaternion-Based Effective Hamiltonian Optimal Control

Enikő Baligács, Nino Wili, José P. Carvalho +2

The paper introduces a quaternion-based optimal control approach to improve dipolar recoupling in magic-angle-spinning solid-state NMR when large chemical shielding anisotropies ar…

quant-ph2026

Quadrature-Symmetric PulsePol for Robust Quantum Control Beyond the Ideal Pulse Approximation

Mayur Jhamnani, Venkata SubbaRao Redrouthu, Jose P. Carvalho +6

PulsePol is an elegantly designed pulse-sequence-based quantum control scheme that enables polarization transfer between electron and nuclear spins, for example, in nitrogen-vacanc…

physics.chem-ph2026

In situ Learning-Based Spin Engineering of Pulsed Dynamic Nuclear Polarization

Filip V. Jensen, José P. Carvalho, Nino Wili +6

Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonan…

physics.chem-ph2026

Extending numerical simulations in SIMPSON: Electron paramagnetic resonance, dynamic nuclear polarisation, propagator splitting, pulse transients, and quadrupolar cross terms

David L. Goodwin, Jose P. Carvalho, Anders B. Nielsen +4

Aimed at the simulation, design, and interpretation of advanced pulse experiments crossing the boundaries between nuclear magnetic resonance (NMR) and electron paramagnetic resonan…

quant-ph2025

Longitudinal Pulsed Dynamic Nuclear Polarization Transfer via Periodic Optimal Control

José P. Carvalho, Anders Bodholt Nielsen, David L. Goodwin +2

Taking inspiration from NMR spectroscopy, periodic irradiation schemes have recently shown remarkable performance when implemented into pulsed dynamic nuclear polarization (DNP) se…

physics.chem-ph2025

Controlling Effective Hamiltonians: Broadband Pulsed Dynamic Nuclear Polarization by Constrained Random Walk and Non-linear Optimization

Anders B. Nielsen, Jose P. Carvalho, Nino Wili +5

We present constrained random walk (cRW) and figure of merit (FOM) based non-linear optimization procedures for systematic design and fundamental understanding of magnetic resonanc…