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In Situ Electrochemical SFG/DFG Study of CN-- and Nitrile Adsorption at Au from 1-Butyl-1-methyl-pyrrolidinium Bis(trifluoromethylsulfonyl) Amide Ionic Liquid ([BMP][TFSA]) Containing 4-{2-[1-(2-Cyanoethyl)-1,2,3,4-tetrahydroquinolin-6-yl]diazenyl} Benzonitrile (CTDB) and K[Au(CN)]
Benedetto Bozzini, Bertrand Busson, Audrey Gayral +4
In this paper we report an in situ electrochemical Sum-/Difference Frequency Generation (SFG/DFG) spectroscopy investigation of the adsorption of nitrile and CN -- from the ionic l…
Non-Uniqueness of Parameters Extracted from Resonant Second-Order Nonlinear Optical Spectroscopies
Bertrand Busson, Abderrahmane Tadjeddine
Experimental data from second-order nonlinear optical spectroscopies (SFG, DFG, and SHG) provide parameters relevant to the physical chemistry of interfaces and thin films. We show…
Nonlinear optical response of a gold surface in the visible range: A study by two-color sum-frequency generation spectroscopy. II. Model for metal nonlinear susceptibility
Bertrand Busson, Laetitia Dalstein
We present a modeling of the nonlinear optical response of a metal surface in order to account for recent experimental results from two-color Sum-Frequency Generation experiments o…