4 papers
Nonlinear reversal of photo-excitation on the attosecond time scale improves ultrafast x-ray diffraction images
Anatoli Ulmer, Phay J. Ho, Bruno Langbehn +28
The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectros…
Attosecond X-ray Core-level Chronoscopy of Aromatic Molecules
Jia-Bao Ji, Zhaoheng Guo, Taran Driver +32
Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalizatio…
Spectrotemporal shaping of attosecond x-ray pulses with a fresh-slice free-electron laser
River R. Robles, Kirk A. Larsen, David Cesar +14
We propose a scheme allowing coherent shaping, i.e., controlling both the amplitude and phase, of attosecond x-ray pulses at free-electron lasers. We show that by seeding an FEL wi…
Attosecond Coherent Electron Motion in a Photoionized Aromatic Molecule
Taran Driver, Zhaoheng Guo, Erik Isele +50
In molecular systems, the ultrafast motion of electrons initiates the process of chemical change. Tracking this electronic motion across molecules requires coupling attosecond time…