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Relaxation dynamics in excited helium nanodroplets probed with high resolution, time-resolved photoelectron spectroscopy
A. C. LaForge, J. D. Asmussen, B. Bastian +18
Superfluid helium nanodroplets are often considered as transparent and chemically inert nanometer-sized cryo-matrices for high-resolution or time-resolved spectroscopy of embedded…
Diffraction imaging of light induced dynamics in xenon-doped helium nanodroplets
Bruno Langbehn, Yevheniy Ovcharenko, Andrew Clark +23
We have explored the light induced dynamics in superfluid helium nanodroplets with wide-angle scattering in a pump-probe measurement scheme. The droplets are doped with xenon atoms…
Collective enhancement of above threshold ionization by resonantly excited helium nanodroplets
R. Michiels, M. Abu-samha, L. B. Madsen +18
Clusters and nanodroplets hold the promise of enhancing high-order nonlinear optical effects due to their high local density. However, only moderate enhancement has been demonstrat…
Evolution and ion kinetics of a XUV-induced nanoplasma in ammonia clusters
R. Michiels, A. C. LaForge, M. Bohlen +14
High-intensity extreme ultraviolet (XUV) pulses from a free-electron laser can be used to create a nanoplasma in clusters. In Ref. [Michiels et al. PCCP, 2020; 22: 7828-7834] we in…
Ultrafast relaxation of photoexcited superfluid He nanodroplets
M. Mudrich, A. LaForge, F. Stienkemeier +21
The relaxation of photoexcited nanosystems is a fundamental process of light-matter interaction. Depending on the couplings of the internal degrees of freedom, relaxation can be ul…
Collective Autoionization in Multiply-Excited Systems: A novel ionization process observed in Helium Nanodroplets
A. C. LaForge, M. Drabbels, N. Brauer +19
Free electron lasers (FELs) offer the unprecedented capability to study reaction dynamics and image the structure of complex systems. When multiple photons are absorbed in complex…