activity
20162026
most citedOptical Imaging of Surface Chemistry and Dynamics in Confinement

122 citations · 186 across the 7 of their papers we have counts for

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physics.chem-ph2026

Collective Electronic Polarization Drives Charge Asymmetry at Oil-Water Interfaces

Gabriele Amante, Klaudia Mrazikova, Gabriele Centi +3

Why kinetically stable oil droplets in water spontaneously acquire a negative charge remains one of the most vigorously debated questions in interfacial science. Here, we combine n…

physics.chem-ph2022★ 10 cited

3D confinement of water: H2O exhibits long-range (> 50 nm) structure while D2O does not

N. Dupertuis, O. B. Tarun, C. Lütgebaucks +1

Water is the liquid of life, thanks to its three-dimensional adaptive hydrogen (H)-bond network. Confinement of this network may lead to dramatic structural changes that influence…

physics.chem-ph2022

Charge gradients around dendritic voids cause nanoscale inhomogeneities in liquid water

Tereza Schonfeldova, Nathan Dupertuis, Yixing Chen +5

Water is the matrix of life and is generally considered a homogeneous, uniform, liquid. Recent experiments report that water is instead a two-state liquid. However, subsequently, t…

physics.chem-ph2020

Vibrational sum frequency scattering in absorptive media: A theoretical case study of nano-objects water

Sergey Kulik, Saranya Pullanchery, Sylvie Roke

The structures of interfaces of nano- and microscale objects in aqueous solution are important for a wide variety of physical, chemical and biological processes. Vibrational sum fr…

physics.chem-ph2017★ 122 cited

Optical Imaging of Surface Chemistry and Dynamics in Confinement

Carlos Macias-Romero, Igor Nahalka, Halil I. Okur +1

The interfacial structure and dynamics of water in a microscopically confined geometry is imaged in three dimensions and on millisecond time scales. We developed a 3D wide-field se…

physics.chem-ph2017★ 4 cited

Generalized expressions for hyper-Rayleigh scattering from isotropic liquids

Yixing Chen, Sylvie Roke

Generalized expressions for second harmonic scattering from isotropically distributed liquid molecules are derived for arbitrary scattering angles and polarization states.