Role of vibrations on decoherence in molecular spin qubits: The case of [Cu(mnt)${}_2$]${}^{2-}$

Luis Escalera-Moreno, Nicolas Suaud, Alejandro Gaita-Ariño +1

Herein we develop a simple first-principles methodology to determine the modulation that vibrations exert on spin energy levels, a key for the rational design of high-temperature m…