Coherent control of nuclear spin isomers of molecules: The role of molecular motion

Abstract

Molecular center-of-mass motion is taken into account in the theory of coherent control of nuclear spin isomers of molecules. It is shown that infrared radiation resonant to the molecular rovibrational transition can substantially enrich nuclear spin isomers and speed up their conversion rate.

arXiv commentREVTEX, 13 pages + 3 eps figures

References in corpus (2)

• New access to very weak interactions in molecules
• Coherent control of enrichment and conversion of molecular spin isomers