Stabilization of charge ordering in La_(1/3)Sr_(2/3)FeO_(3-d) by magnetic exchange

Abstract

The magnetic exchange energies in charge ordered La_(1/3)Sr_(2/3)FeO_(3-d) (LSFO) and its parent compound LaFeO_(3) (LFO) have been determined by inelastic neutron scattering. In LSFO, the measured ratio of ferromagnetic exchange between Fe3+ - Fe5+ pairs (J_F) and antiferromagnetic exchange between Fe3+ - Fe3+ pairs (J_AF) fulfills the criterion for charge ordering driven by magnetic interactions (|J_F/J_AF| > 1). The 30% reduction of J_AF as compared to LFO indicates that doped holes are delocalized, and charge ordering occurs without a dominant influence from Coulomb interactions.

arXiv comment18 pages, 4 color figures

References in corpus (3)

• Magnetic neutron scattering study of YVO3: Evidence for an orbital Peierls state
• Implications of Charge Ordering for Single-Particle Properties of High-Tc Superconductors
• Investigation of the presence of charge order in magnetite by measurement of the spin wave spectrum

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