Lattice dynamics and phonon softening in Ni-Mn-Al Heusler alloys

Abstract

Inelastic and elastic neutron scattering have been used to study a single crystal of the Ni${}_{54}$Mn${}_{23}$Al${}_{23}$ Heusler alloy over a broad temperature range. The paper reports the first experimental determination of the low-lying phonon dispersion curves for this alloy system. We find that the frequencies of the TA${}_2$ modes are relatively low. This branch exhibits an anomaly (dip) at a wave number ${\xi }_0=1/3\approx 0.33$, which softens with decreasing temperature. Associated with this anomalous dip at ${\xi }_0$, an elastic central peak scattering is also present. We have also observed satellites due to the magnetic ordering.

6 pages, 6 figures. Accepted for publication in the Physical Review B

References in corpus (6)

• First-principles study of lattice instabilities in the ferromagnetic martensite Ni${}_2$MnGa
• Premartensitic transition driven by magnetoelastic interaction in bcc ferromagnetic $N{i}_{2}MnGa$
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• Strain and order-parameter coupling in Ni-Mn-Ga Heusler alloys from resonant ultrasound spectroscopy
• Determination of the vibrational contribution to the entropy change at the martensitic transformation in Ni-Mn-Sn metamagnetic shape memory alloys: A combined approach of time-of-flight neutron spectroscopy and ab-initio calculations
• Strain behavior and lattice dynamics in Ni50Mn35In15