Evolution of spin-wave excitations in ferromagnetic metallic manganites

Abstract

Neutron scattering results are presented for spin-wave excitations of three ferromagnetic metallic $A_{1-x}{A}_x^{\prime }$MnO${}_3$ manganites (where $A$ and $A^{\prime }$ are rare- and alkaline-earth ions), which when combined with previous work elucidate systematics of the interactions as a function of carrier concentration $x$, on-site disorder, and strength of the lattice distortion. The long wavelength spin dynamics show only a very weak dependence across the series. The ratio of fourth to first neighbor exchange ($J_4/J_1$) that controls the zone boundary magnon softening changes systematically with $x$, but does not depend on the other parameters. None of the prevailing models can account for these behaviors.

Submitted to Phys. Rev. Lett