Time and length scales in supercooled liquids
arXiv:cond-mat/0310210 · doi:10.1103/PhysRevE.69.020201
Abstract
We numerically obtain the first quantitative demonstration that development of spatial correlations of mobility as temperature is lowered is responsible for the ``decoupling'' of transport properties of supercooled liquids. This result further demonstrates the necessity of a spatial description of the glass formation and therefore seriously challenges a number of popular alternative theoretical descriptions.
4 pages, 4 figs; improved version: new refs and discussions
References in corpus (5)
- Geometrical explanation and scaling of dynamical heterogeneities in glass forming systems
- Coarse-grained microscopic model of glass formers
- Real space origin of temperature crossovers in supercooled liquids
- Non-topographic description of inherent structure dynamics in glass formers
- Finite size scaling analysis of the glass transition
Cited by in corpus (115)
- Theoretical perspective on the glass transition and amorphous materials
- Direct experimental evidence of a growing length scale accompanying the glass transition
- The Physics of the Colloidal Glass Transition
- Dynamics on the Way to Forming Glass: Bubbles in Space-time
- On the Adam-Gibbs-Wolynes scenario for the viscosity increase in glasses
- Universal nature of particle displacements close to glass and jamming transitions
- Bond orientational ordering in liquids: Towards a unified description of water-like anomalies, liquid-liquid transition, glass transition, and crystallization
- Inhomogeneous Mode-Coupling Theory and Growing Dynamic Length in Supercooled Liquids
- On the Rigidity of Amorphous Solids
- What do we learn from the shape of the dynamical susceptibility of glass-formers?
- Dynamical Heterogeneity close to the Jamming Transition in a Sheared Granular Material
- Spatial correlations in the dynamics of glassforming liquids: Experimental determination of their temperature dependence
- Spontaneous and induced dynamic fluctuations in glass-formers I: General results and dependence on ensemble and dynamics
- Dynamic heterogeneity in amorphous materials
- Excitation lines and the breakdown of Stokes-Einstein relations in supercooled liquids
- Fractional Stokes-Einstein and Debye-Stokes-Einstein relations in a network forming liquid
- Length scale for the onset of Fickian diffusion in supercooled liquids
- Dynamic criticality in glass-forming liquids
- Diverging length scale and upper critical dimension in the Mode-Coupling Theory of the glass transition
- Spontaneous and induced dynamic correlations in glass-formers II: Model calculations and comparison to numerical simulations
- Non-linear susceptibility in glassy systems: a probe for cooperative dynamical length scales
- Length scale dependence of dynamical heterogeneity in a colloidal fractal gel
- The Monte-Carlo dynamics of a binary Lennard-Jones glass-forming mixture
- Velocity correlations in dense granular flows
- Relaxation in a glassy binary mixture: Comparison of the mode-coupling theory to a Brownian dynamics simulation
- Clustering and heterogeneous dynamics in a kinetic Monte-Carlo model of self-propelled hard disks
- Relaxation and physical aging in network glasses: a review
- Structural relaxation of polydisperse hard spheres: comparison of the mode-coupling theory to a Langevin dynamics simulation
- Scaling properties of granular rheology near the jamming transition
- Coupling/decoupling between translational and rotational dynamics in a supercooled molecular liquid
- Dynamical Exchanges in Facilitated Models of Supercooled liquids
- Lengthscale dependence of dynamic four-point susceptibilities in glass formers
- Heterogeneity and growing lengthscales in the dynamics of kinetically constrained lattice gases in two dimensions
- Dynamic heterogeneity in a glass forming fluid: susceptibility, structure factor and correlation length
- De-coupling of Exchange and Persistence Times in Atomistic Models of Glass Formers
- Temperature dependence of spatially heterogeneous dynamics in a model of viscous silica
- Finite size effects in the dynamics of glass-forming liquids
- One micron length scale controls kinetic stability of low energy glasses
- Multiple length and time scales of dynamic heterogeneities in model glass-forming liquids: A systematic analysis of multi-point and multi-time correlations
- An introduction to the colloidal glass transition
- Critical fluctuations and breakdown of Stokes-Einstein relation in the Mode-Coupling Theory of glasses
- Analysis of a growing dynamic length scale in a glass-forming binary hard-sphere mixture
- Microscopic dynamics of supercooled liquids from first principles
- Connections of activated hopping processes with the breakdown of the Stokes-Einstein relation and with aspects of dynamical heterogeneities
- Dynamics and structure of an aging binary colloidal glass
- Short-time -relaxation in glass-forming liquids is cooperative in nature
- Growing length and time scales in a suspension of athermal particles
- Anomalous diffusion of driven particles in supercooled liquids
- Revisiting the slow dynamics of a silica melt using Monte Carlo simulations
- Preparation and relaxation of very stable glassy states of a simulated liquid
- Microscopic Structural Relaxation in a Sheared Supercooled Colloidal Liquid
- Can the glass transition be explained without a growing static length scale?
- Multi-time density correlation functions in glass-forming liquids: Probing dynamical heterogeneity and its lifetime
- Fluctuations in glassy systems
- Mechanisms of bulk and surface diffusion in metallic glasses determined from molecular dynamics simulations
- Length scale dependence of the Stokes-Einstein and Adam-Gibbs relations in model glass formers
- Cooperative Behavior of Kinetically Constrained Lattice Gas Models of Glassy Dynamics
- Liquid-liquid transition revealed by quasi-static cooling of an ultra-viscous metallic liquid
- On the critical behavior of the specific heat in glass-formers
- Free-then-freeze: transient learning degrees of freedom for introducing function in materials
- Fundamental Theory of Statistical Particle Dynamics
- Length scales in Brownian yet non-Gaussian dynamics
- Decoupling phenomena in supercooled liquids: Signatures in the energy landscape
- Fluctuations in the coarsening dynamics of the O(N) model: are they similar to those in glassy systems?
- Dynamical Heterogeneity in Lattice Glass Models
- Fickian crossover and lengthscales from two point functions in supercooled liquids
- Dynamical heterogeneity in a highly supercooled liquid: Consistent calculations of correlation length, intensity, and lifetime
- Multiple time scales hidden in heterogeneous dynamics of glass-forming liquids
- Non-equilibrium dynamics of spin facilitated glass models
- Criticality and correlated dynamics at the irreversibility transition in periodically driven colloidal suspensions
- Dynamical heterogeneity in aging colloidal glasses of Laponite
- Growing dynamical length, scaling and heterogeneities in the 3d Edwards-Anderson model
- Lifetime of dynamic heterogeneity in strong and fragile kinetically constrained spin models
- Anisotropic spatially heterogeneous dynamics on the and relaxation time scales studied via a four-point correlation function
- Analysis of cooperativity and localization for atomic rearrangements
- Diverging length scale of the inhomogeneous mode-coupling theory: a numerical investigation
- Static correlations functions and domain walls in glass-forming liquids: the case of a sandwich geometry
- Dynamical Heterogeneity in a Highly Supercooled Liquid under a Sheared Situation
- Coarse-grained Soft-Clusters Remain non-Diffusing in the Melt State
- Intermittent relaxation and avalanches in extremely persistent active matter
- Anisotropic spatially heterogeneous dynamics in a model glass-forming binary mixture
- Heterogeneous dynamics and its length scale in simple ionic liquid models: A computational study
- Yield stress in amorphous solids: A mode-coupling theory analysis
- Classification of mobile- and immobile-molecule timescales for the Stokes-Einstein and Stokes-Einstein-Debye relations in supercooled water
- Divergent four-point dynamic density correlation function of a glassy colloidal suspension: a diagrammatic approach
- Aging of rotational diffusion in colloidal gels and glasses
- Analytical Calculation of Four-Point Correlations for a Simple Model of Cages Involving Numerous Particles
- Is there a fractional breakdown of the Stokes-Einstein relation in Kinetically Constrained Models at low temperature?
- Dynamical heterogeneity in a glass forming ideal gas
- Reduced strength and extent of dynamic heterogeneity in a strong glass former as compared to fragile glass formers
- Crossover from stationary to aging regime in glassy dynamics
- Inherent Structures and Kauzmann Temperature of Confined Liquids
- Factors correlating to enhanced surface diffusion in metallic glasses
- Distributions of pore sizes and atomic densities in binary glasses revealed by molecular dynamics simulations
- Theoretical analysis for critical fluctuations of relaxation trajectory near a saddle-node bifurcation
- Experimental search for dynamic heterogeneities in molecular glass formers
- Dynamic Length Scales in Glass-Forming Liquids: A Inhomogeneous Molecular Dynamics Simulation Approach
- Are supercooled liquids Fickian yet non Gaussian?
- Connecting Relaxation Time to a Dynamical Length Scale in Athermal Active Glass Formers
- Continuous time random walk concepts applied to extended mode coupling theory: A study of the Stokes-Einstein breakdown
- Collective motion of macroscopic spheres floating on capillary ripples: Dynamic heterogeneity and dynamic criticality
- Characterising the slow dynamics of the swap Monte Carlo algorithm
- Finite-size scaling for non-linear rheology of fluids confined in a small space
- Automated characterization of spatial and dynamical heterogeneity in supercooled liquids via implementation of Machine Learning
- A numerical study of longtime dynamics and ergodic-nonergodic transitions in dense simple fluids
- Molecular motion at the experimental glass transition
- Collisional Statistics and Dynamics of 2D Hard-Disk Systems: From Fluid to Solid
- Delocalization transition of a small number of particles in a box with periodic boundary conditions
- Displacement correlations in a two-dimensional colloidal liquid and their relationship with shear strain correlations
- Melting Transition of Vortex Lattice in Point Vortex Systems
- Microfluidic velocimetry reveals spatial cooperativity in soft glassy flows
- Subdiffusive motion in kinetically constrained models
- Microscopic Theory of a Fluctuation-Induced Dynamical Crossover in Supercooled Liquids
- Relation between dynamic heterogeneities observed in scattering experiments and four-body correlations
- Cooperative jump motions of jammed particles in a one-dimensional periodic potential