Momentum-space engineering in van der Waals heterostructures

Abstract

Twenty years of graphene research have established Dirac fermions as a versatile platform for exploring quantum topological phenomena. Yet control over graphene's low-energy spectrum mostly follows the route of miniband engineering using real-space superlattices. Here we introduce a complementary approach based on momentum-space 'Umklapp' band engineering. This is realised by matching reciprocal space positions of band edges of two adjacent highly incommensurate 2D crystals to coincide upon a boost from their Bragg vectors, creating resonant interlayer hybridisation that qualitatively reconstructs their spectra. To demonstrate this approach experimentally, we use monolayer graphene on MoS${}_2$, twisted such that MoS${}_2$ Q-valley states are brought by Umklapp into energy-momentum resonance with graphene's Dirac cones. The ensuing hybridization results in the formation of a clear additional Dirac-like spectral feature, identified by a distinct Landau-level fan and Shubnikov-de Haas oscillations characteristic to Berry phase $\pi$ electrons. These new topological spectral features create a spin-valley locked Ising system which is robust against small twist-angle variations that can be further tuned by an external displacement field. More broadly, Umklapp band engineering offers a practical strategy for tailoring the electronic structure in van der Waals heterostructures, expanding the design space of quantum materials beyond moiré superlattices and weak proximity effects.

arXiv comment18 pages 4 figures