Spin-Lattice Dynamics and Interactions in Magnonic Spinels

Abstract

Minimizing magnetic damping while understanding spin-lattice interactions remains a key challenge for magnonics. We show site-specific Al/Li ordering in spinel ferrites drives a ferrimagnetic insulating state, quenching the Fermi-level density of states. \textit{Ab initio} calculations reveal collective acoustic modes alongside sub-lattice-selective optical modes on tetrahedral and octahedral networks, providing a microscopic understanding of substitution-driven spin dynamics. Crucially, the low-frequency magnon and acoustic phonon modes intersect, driving strong hybridization for low-loss technologies.

8 pages and 3 figures