Orbital-geometric spin response: inter-band coherence versus orbital-to-spin conversion

Abstract

Orbitronics seeks to convert orbital angular momentum (OAM) into spin, but its microscopic dynamics is not understood. Here I show that, at moderate spin-orbit coupling, an electrically induced spin density contains a direct term and an \textit{orbital-geometric spin response} (OGSR) due to inter-band coherence of the spinless parent Hamiltonian---related to OAM but not descended from it. In massive Dirac fermions the OGSR survives as the net OAM vanishes, and generates \textit{counterflow}, opposing the direct response. These results provide guidelines for optimising orbitronic systems.