Electronic Structure and Superconductivity in La${}_{1.55}$Sr${}_{0.45}$CuO${}_4$/La${}_2$CuO${}_4$ Artificial High-$T_c$ Superlattices Probed by Hard and Soft X-ray Spectroscopy

Abstract

In La${}_{1.55}$Sr${}_{0.45}$CuO${}_4$/La${}_2$CuO${}_4$ (LSCO/LCO) artificial high-$T_c$ superlattices (AHTS), grown by quantum material design, the superconducting dome can be tuned by varying the geometric ratio $L/d$, where $L$ is the LCO layer thickness and $d$ is the superlattice nanoscale period. Here, we combine hard X-ray photoelectron spectroscopy (HAXPES) and polarization-dependent soft X-ray absorption spectroscopy (XAS) to probe how the electronic structure evolves across the $L/d$-tuned superconducting dome. We observe systematic chemical-potential evolution across the series, together with enhanced spectral weight near the Fermi level, enhanced local and non-local screening signatures, and increased in-plane orbital polarization near the top of the dome. Together, these spectroscopic signatures provide insight into the emergence of Fano-Feshbach resonant superconductivity in the LSCO/LCO AHTS series.